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Ito, Takashi; Higemoto, Wataru; Koda, Akihiro*; Nakamura, Jumpei*; Shimomura, Koichiro*
Interactions (Internet), 245(1), p.25_1 - 25_7, 2024/12
Fujihara, Masayoshi; Okabe, Hirotaka*; Koda, Akihiro*
Interactions (Internet), 245(1), p.13_1 - 13_6, 2024/12
Quantum states are difficult to observe experimentally. In addition, ideal model materials have not been found for some of the lattice systems in which exotic quantum states are predicted to be realized. Numerous candidates for low-dimensional quantum magnets are hidden in copper minerals, and the number of candidates is increasing every year. We succeeded to synthesize seven copper minerals by imitating the environment where they are discovered and reported their quantum states. The properties of pulsed muons are very suitable for investigating the spin state of artificial copper minerals.
Shimomura, Koichiro*; Koda, Akihiro*; Pant, A. D.*; Sunagawa, Hikaru*; Fujimori, Hiroshi*; Umegaki, Izumi*; Nakamura, Jumpei*; Fujihara, Masayoshi; Tampo, Motonobu*; Kawamura, Naritoshi*; et al.
Interactions (Internet), 245(1), p.31_1 - 31_6, 2024/12
Maruyama, Shuhei; Yamamoto, Akio*; Endo, Tomohiro*
Annals of Nuclear Energy, 205, p.110591_1 - 110591_13, 2024/09
Abe, Satoshi; Shibamoto, Yasuteru
Annals of Nuclear Energy, 202, p.110461_1 - 110461_16, 2024/07
Times Cited Count:0Nakamichi, Shinya; Sunaoshi, Takeo*; Hirooka, Shun; Vauchy, R.; Murakami, Tatsutoshi
Journal of Nuclear Materials, 595, p.155072_1 - 155072_11, 2024/07
Frazer, D.*; Saleh, T. A.*; Matsumoto, Taku; Hirooka, Shun; Kato, Masato; McClellan, K.*; White, J. T.*
Nuclear Engineering and Design, 423, p.113136_1 - 113136_7, 2024/07
Nanoindentation based techniques can be employed on minute volumes of material to measure mechanical properties, including Young's modulus, hardness, and creep stress exponents. In this study, (U,Ce)O solid solutions samples are used to develop elevated temperature nanoindentation and nanoindentation creep testing methods for use on mixed oxide fuels. Nanoindentation testing was performed on 3 separate (Ux-1,Cex)O compounds ranging from x equals 0.1 to 0.3 at up to 800 C: their Young's modulus, hardness, and creep stress exponents were evaluated. The Young's modulus decreases in the expected linear manner while the hardness decreases in the expected exponential manner. The nanoindentation creep experiments at 800 C give stress exponent values, n=4.7-6.9, that suggests dislocation motion as the deformation mechanism.
Li, L.*; Miyamoto, Goro*; Zhang, Y.*; Li, M.*; Morooka, Satoshi; Oikawa, Katsunari*; Tomota, Yo*; Furuhara, Tadashi*
Journal of Materials Science & Technology, 184, p.221 - 234, 2024/06
Times Cited Count:0 Percentile:0(Materials Science, Multidisciplinary)Sato, Ikken; Yoshikawa, Shinji; Yamashita, Takuya; Shimomura, Kenta; Cibula, M.*; Mizokami, Shinya*
Nuclear Engineering and Design, 422, p.113088_1 - 113088_24, 2024/06
Sato, Yuki; Kakuto, Takeshi*; Tanaka, Takayuki*; Shimano, Hiroyuki*; Morohashi, Yuko; Hatakeyama, Tomoyoshi*; Nakajima, Junsaku; Ishiyama, Masahiro
Nuclear Instruments and Methods in Physics Research A, 1063, p.169300_1 - 169300_7, 2024/06
Nguyen, B. V. C.*; Murakami, Kenta*; Chena, L.*; Phongsakorn, P. T.*; Chen, X.*; Hashimoto, Takashi; Hwang, T.*; Furusawa, Akinori; Suzuki, Tatsuya*
Nuclear Materials and Energy (Internet), 39, p.101639_1 - 101639_9, 2024/06
Collaborative Laboratories for Advanced Decommissioning Science; Shinshu University*
JAEA-Review 2023-053, 87 Pages, 2024/05
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2022. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Development of environmental mitigation technology with novel water purification agents" conducted from FY2020 to FY2022. The present study aims to develop a reusable adsorbent for strontium ions with high adsorption property to contribute to the improvement of the treatment process of radioactive contaminated water generated by the Great East Japan Earthquake. As a result, reusable adsorbent materials showing excellent Sr adsorption performances were developed. The current adsorbent materials for strontium are extremely expensive and single use, so the storage and disposal of massive generation of waste have become a major problem.
Collaborative Laboratories for Advanced Decommissioning Science; i-Lab*
JAEA-Review 2023-029, 77 Pages, 2024/05
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2022. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Challenge to advancement of debris composition and direct isotope measurement by microwave-enhanced LIBS" conducted from FY2020 to FY2022. The present study aims to increase the emission intensity of LIBS (laser-induced breakdown spectroscopy) by superimposing MW (microwave) and apply it to uranium isotope measurement. In FY2022, we improved the cooling method and reduce unnecessary functions in of the semiconductor microwave oscillator, and apply the optimized conditions obtained from simulations to the LIBS experiment for the microwave antenna gave better results.
Sun, Haomin; Kunugi, Tomoaki*; Yokomine, Takehiko*; Shen, X.*; Hibiki, Takashi*
Experimental Thermal and Fluid Science, 154, p.111171_1 - 111171_24, 2024/05
Times Cited Count:0Ishikado, Motoyuki*; Takahashi, Ryuta*; Yamauchi, Yasuhiro*; Nakamura, Masatoshi*; Ishimaru, Sora*; Yamauchi, Sara*; Kawamura, Seiko; Kira, Hiroshi*; Sakaguchi, Yoshifumi*; Watanabe, Masao; et al.
JPS Conference Proceedings (Internet), 41, p.011010_1 - 011010_7, 2024/05
Omer, M.; Shizuma, Toshiyuki*; Hajima, Ryoichi*; Koizumi, Mitsuo
Journal of Applied Physics, 135(18), p.184903_1 - 184903_10, 2024/05
Miyazaki, Kanako*; Takehara, Masato*; Minomo, Kenta*; Horie, Kenji*; Takehara, Mami*; Yamasaki, Shinya*; Saito, Takumi*; Onuki, Toshihiko*; Takano, Masahide; Shiotsu, Hiroyuki; et al.
Journal of Hazardous Materials, 470(15), p.134104_1 - 134104_11, 2024/05
Micheau, C.; Ueda, Yuki; Motokawa, Ryuhei; Akutsu, Kazuhiro*; Yamada, Norifumi*; Yamada, Masako*; Moussaoui, S. A.*; Makombe, E.*; Meyer, D.*; Berthon, L.*; et al.
Journal of Molecular Liquids, 401, p.124372_1 - 124372_12, 2024/05
Supramolecular organization of extractant molecules impacts metal ions separation behavior. Probing bulk and interfacial structures of the relevant systems is expected to provide key insights into the metal ion selectivity and kinetic aspects. The supramolecular features of two solvent extraction systems based on malonamide extractants THMA in toluene and DBMA in n-heptane were studied using small-angle X-ray scattering for the organic bulk phases, as well as interfacial tension and neutron reflectivity measurements for the interfaces. In the bulk solution, THMA forms dimeric/trimeric associates but no aggregates in toluene, while DBMA forms large aggregates in n-heptane. On the other hand, THMA accumulates in a diffuse layer at the interface at high THMA concentration, whereas DBMA forms a compact but thinner layer. After Pd(II) extraction, the thickness of interfacial layers decreases in the case of THMA, and totally vanishes in the case of DBMA. Based on these new structural information, two mechanisms are proposed for Pd(II) and Nd(III) extraction with malonamides. In toluene, THMA associates slightly accumulate in the vicinity of the interface, then coordinate Pd(II) and diffuse into the organic bulk phase. In n-heptane, DBMA aggregates adsorb at the interface then pick up Nd(III) cations in their polar cores and finally diffuse into the bulk.
Kato, Masato; Oki, Takumi; Watanabe, Masashi; Hirooka, Shun; Vauchy, R.; Ozawa, Takayuki; Uwaba, Tomoyuki; Ikusawa, Yoshihisa; Nakamura, Hiroki; Machida, Masahiko
Journal of the American Ceramic Society, 107(5), p.2998 - 3011, 2024/05
Times Cited Count:0 Percentile:0.01(Materials Science, Ceramics)Takata, Hyoe*; Wakiyama, Yoshifumi*; Wada, Toshihiro*; Hirao, Shigekazu*; Aono, Tatsuo*; Nakanishi, Takahiro; Misono, Toshiharu; Shiribiki, Takehiko; Aoyama, Michio*
Marine Chemistry, 262, p.104384_1 - 104384_6, 2024/05